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Surface coatings and patterning technologies are essential for variousphysicochemical applications. In this Letter, we describe key parameters toachieve uniform particle coatings from binary solutions: First, multiplesequential Marangoni flows, set by solute and surfactant simultaneously,prevent non-uniform particle distributions and continuously mix suspendedmaterials during droplet evaporation. Second, we show the importance ofparticle-surface interactions that can be established by surface-adsorbedmacromolecules. To achieve a uniform deposit in a binary mixture, a smallconcentration of surfactant and surface-adsorbed polymer (0.05 wt% each) issufficient, which offers a new physicochemical avenue for control of coatings.

Controlled uniform coating from the interplay of Marangoni flows and surface-adsorbed macromolecules