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A rational approach to identify polyatomic molecules that appear to bepromising candidates for direct Doppler cooling with lasers is outlined.First-principle calculations for equilibrium structures and Franck--Condonfactors of selected representatives with different point-group symmetries(including chiral non-symmetric group C$_1$) have been performed and highpotential for laser-cooling of these molecules is indicated.

Polyatomic candidates for cooling of molecules with lasers from simple theoretical concepts