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Using resonant soft x-ray scattering as a function of both temperature andmagnetic field, we reveal a large number of almost degenerate magnetic ordersin SrCo6O11. The Ising-like spins in this frustrated material in fact exhibit aso-called magnetic devil's staircase. It is demonstrated how a magnetic fieldinduces transitions between different microscopic spin configurations, which isresponsible for the magnetoresistance of SrCo6O11. This material thereforeconstitutes a unique combination of a magnetic devil's staircase and spin valveeffects, yielding a novel type of magnetoresistance system.

Observation of Devil's Staircase in the Novel Spin Valve System SrCo$_6$O$_{11}$