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The effective moment of inertia of a CO impurity molecule in 4HeN and p-(H2)N solvent clusters initially increases with N but then commences a nonclassical decrease at N=4 (4He) or N=6 (p-H2). This suggests molecule-solvent decoupling and a transition to microscopic superfluidity. However, the quantum decoupling mechanism has not been elucidated. To understand the decoupling mechanism, a one-dimensional model is introduced in which the 4He atoms are confined to a ring. This model captures the physics and shows that decoupling happens primarily because of bosonic solvent-solvent repulsion. Quantum Monte Carlo and basis set calculations suggest that the system can be modeled as a stirred Tonks-Girardeau gas. This allows the N-particle time-dependent Schrödinger equation to be solved directly. Computations of the integrated particle current reveal a threshold for stirring and current generation, indicative of superfluidity.

physical review letters

Microscopic Superfluidity in<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>He</mml:mi></mml:mrow><mml:mprescripts /><mml:none /><mml:mrow><mml:mn>4</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math>Clusters Stirred by a Rotating Impurity Molecule

Microscopic Superfluidity inHe4Clusters Stirred by a Rotating Impurity Molecule