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Magnetization, nuclear magnetic resonance, high-resolution x-ray diffractionand magnetic field-dependent neutron diffraction measurements reveal a novelmagnetic ground state of Ba{0.60}K{0.40}Mn2As2 in which itinerantferromagnetism (FM) below a Curie temperature TC = 100 K arising from the dopedconduction holes coexists with collinear antiferromagnetism (AFM) of the Mnlocal moments that order below a Neel temperature TN = 480 K. The FM orderedmoments are aligned in the tetragonal ab-plane and are orthogonal to theAFM-ordered Mn moments that are aligned along the c-axis. The magnitude andnature of the low-T FM ordered moment correspond to complete polarization ofthe doped-hole spins (half-metallic itinerant FM) as deduced from magnetizationand ab-plane electrical resistivity measurements.

Coexistence of Half-Metallic Itinerant Ferromagnetism with Local-Moment Antiferromagnetism in Ba{0.60}K{0.40}Mn2As2