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International audienceWe report integral cross sections for the S(1D2)+HD(j=0)→DS+H and HS+D reaction channels obtained through crossed-beam experiments reaching collision energies as low as 0.46 meV and from adiabatic time-independent quantum-mechanical calculations. While good overall agreement with experiment at energies above 10 meV is observed, neither the product channel branching ratio nor the low-energy resonancelike features in the HS+D channel can be theoretically reproduced. A nonadiabatic treatment employing highly accurate singlet and triplet potential energy surfaces is clearly needed to resolve the complex nature of the reaction dynamics

physical review letters

Dynamics of the<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi mathvariant="bold">S</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mmultiscripts><mml:mi>D</mml:mi><mml:mn>2</mml:mn><mml:none /><mml:mprescripts /><mml:none /><mml:mn>1</mml:mn></mml:mmultiscripts><mml:mo stretchy="false">)</mml:mo><mml:mo mathvariant="bold">+</mml:mo><mml:mi>HD</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mi>j</mml:mi><mml:mo mathvariant="bold">=</mml:mo><mml:mn>0</mml:mn><…

Dynamics of theS(D21)+HD(j=0<…