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The Faraday rotation and magneto-optical absorption spectral measurementswere conducted to reveal the full-magnetization process and map out a magneticphase diagram of a typical geometrical frustrated magnet, ZnCr2O4, by using theelectromagnetic flux compression method in ultra-magnetic fields up to 600 T. Afully polarized ferromagnetic phase is observed in which the absorption spectraassociated with an exciton-magnon-phonon transition disappears. Furthermore,prior to the fully polarized ferromagnetic phase above 410 T, we found a novelmagnetic phase above 350 T followed by a canted 3:1 phase.

Magnetic phases of a highly frustrated magnet, ZnCr2O4, up to an ultra-high magnetic field of 600 T