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Dielectric loss spectra covering 13 decades in frequency were collected for2-ethyl-1-hexanol, a monohydroxy alcohol that exhibits a prominent Debye-likerelaxation, typical for several classes of hydrogen-bonded liquids. The thermalvariation of the dielectric absorption amplitude agrees well with that of thehydrogen-bond equilibrium population, experimentally mapped out using nearinfrared (NIR) and nuclear magnetic resonance (NMR) measurements. Despite thisagreement, temperature-jump NIR spectroscopy reveals that the hydrogen-bondswitching rate does not define the frequency position of the prominentabsorption peak. This contrasts with widespread notions and models basedthereon, but is consistent with a recent approach.

Hydrogen-bond equilibria and life times in a supercooled monohydroxy alcohol