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We report the successful extraction of spin polarized current from theorganic-based room temperature ferrimagnetic semiconductor V[TCNE]x (x~2, TCNE:tetracyanoethylene; TC ~ 400 K, EG ~ 0.5 eV, s ~ 10-2 S/cm) and its subsequentinjection into a GaAs/AlGaAs light-emitting diode (LED). The spin currenttracks the magnetization of V[TCNE]x~2, is weakly temperature dependent, andexhibits heavy hole / light hole asymmetry. This result has implications forroom temperature spintronics and the use of inorganic materials to probe spinphysics in organic and molecular systems.

Electrical spin injection from an organic-based ferrimagnet in a hybrid organic/inorganic heterostructure