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Electron spin qubits in molecular systems offer high reproducibility and theability to self assemble into larger architectures. However, interactionsbetween neighbouring qubits are 'always-on' and although the electron spincoherence times can be several hundred microseconds, these are still muchshorter than typical times for nuclear spins. Here we implement anelectron-nuclear hybrid scheme which uses coherent transfer between electronand nuclear spin degrees of freedom in order to both controllably turn on/offdipolar interactions between neighbouring spins and benefit from the longnuclear spin decoherence times (T2n). We transfer qubit states between theelectron and 15N nuclear spin in 15N@C60 with a two-way process fidelity of88%, using a series of tuned microwave and radiofrequency pulses and measure anuclear spin coherence lifetime of over 100 ms.

Coherent state transfer between an electron- and nuclear spin in 15N@C60