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A molecular level analysis of segmental trajectories obtained from moleculardynamics simulations is used to obtain the full relaxation time spectrum inaging polymer glasses subject to three different deformation protocols. As inexperiments, dynamics can be accelerated by several orders of magnitude, and anarrowing of the distribution of relaxation times during creep is directlyobserved. Additionally, the acceleration factor describing the transformationof the relaxation time distributions is computed and found to obey a universaldependence on the global strain, independent of age and deformation protocol.

A microscopic view of accelerated dynamics in deformed polymer glasses