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Huge deformations of the crystal lattice can be achieved in materials withinherent structural instability by epitaxial straining. By coherent growth onseven different substrates the in-plane lattice constants of 50 nm thickFe70Pd30 films are continuously varied. The maximum epitaxial strain reaches8,3 % relative to the fcc lattice. The in-plane lattice strain results in aremarkable tetragonal distortion ranging from c/abct = 1.09 to 1.39, coveringmost of the Bain transformation path from fcc to bcc crystal structure. Thishas dramatic consequences for the magnetic key properties. Magnetometry andX-ray circular dichroism (XMCD) measurements show that Curie temperature,orbital magnetic moment, and magnetocrystalline anisotropy are tuned over broadranges.

Tuning of crystal structure and magnetic properties by exceptionally large epitaxial strains