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I investigate energy transfer in a donor-acceptor pair beyond weaksystem-bath coupling. I identify a transition from coherent to incoherentdynamics with increasing temperature, due to multi-phonon effects not capturedby a standard weak-coupling treatment. The crossover temperature has a markeddependence on the degree of spatial correlation between fluctuationsexperienced at the two system sites. For strong correlations, this leads to thepossibility of coherence surviving into a high temperature regime.

Correlation-dependent coherent to incoherent transitions in resonant energy transfer dynamics