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An ultra-fast quench is applied to binary mixtures of superparamagneticcolloidal particles confined at a two-dimensional water-air interface by asudden increase of an external magnetic field. This quench realizes a virtuallyinstantaneous cooling which is impossible in molecular systems. Usingreal-space experiments, the relaxation behavior after the quench is explored.Local crystallites with triangular and square symmetry are formed on differenttime scales and the correlation peak amplitude of the small particles evolvesnonmonotonically in time in agreement with Brownian dynamics computersimulations.

Ultra-fast quenching of binary colloidal suspensions in an external magnetic field