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The local effect of an interstitial hydrogenlike particle on localized f electrons was studied in PrPb3 by means of micro+ spin rotation and relaxation. Spontaneous micro+ spin precession with harmonic frequencies was observed for the first time in f electron compounds. We demonstrate that the signal is derived from a coupling between the micro+ spin and the hyperfine-enhanced nuclear spin of nearest neighbor (NN) 141Pr with Ising-like anisotropy. The signal also suggests a marked suppression of spin dynamics of the NN 141Pr in comparison with that of the bulk 141Pr. These facts strongly indicate modification of the f electronic state due to the interstitial charged particle.

physical review letters

Quantized Hyperfine Field at an Implanted<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:msup><mml:mi>μ</mml:mi><mml:mo>+</mml:mo></mml:msup></mml:math>Site in<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:msub><mml:mi>PrPb</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:math>: Interplay between Localized<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>f</mml:mi></mml:math>Electrons and an Interstitial …

Quantized Hyperfine Field at an Implantedμ+Site inPrPb3: Interplay between LocalizedfElectrons and an Interstitial …