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Polydispersity is found to have a significant effect on the potential energylandscape; the the average inherent structure energy with temperature decreaseswith polydispersity. Increasing polydispersity at fixed volume fractiondecreases the glass transition temperature and the fragility of glass formationanalogous to the antiplasticization seen in some polymeric melts. Aninteresting temperature dependent crossover of heterogeneity withpolydispersity is observed at low temperature due to the faster build-up ofdynamic heterogeneity at lower polydispersity.

Energy Landscape, Anti-Plasticization and Polydispersity Induced Crossover of Heterogeneity in Supercooled Polydisperse Liquids