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Associative polymers with sticker-and-spacer architectures undergo phasetransitions that combine phase separation and bond percolation. Here, wegeneralize mean-field models for bond percolation and extract effective stickerinteraction strengths from experimental data for specific proteins. We usegraph-based Monte Carlo simulations to evaluate effects ignored by mean-fieldmodels. These include bond cooperativity defined as changes to strengths of newbonds (physical crosslinks) given the presence of a prior bond. We find thatbond cooperativity fundamentally alters phase behavior, especially insub-stoichiometric regimes for valencies of complementary stickers.

Generalized models for bond percolation transitions of associative polymers