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We apply improved nucleon-nucleon potentials up to fifth order in chiraleffective field theory, along with a new analysis of the theoretical truncationerrors, to study nucleon-deuteron (Nd) scattering and selected low-energyobservables in 3H, 4He, and 6Li. Calculations beyond second order differ fromexperiment well outside the range of quantified uncertainties, providing trulyunambiguous evidence for missing three-nucleon forces within the employedframework. The sizes of the required three-nucleon force contributions agreewell with expectations based on Weinberg's power counting. We identify theenergy range in elastic Nd scattering best suited to study three-nucleon forceeffects and estimate the achievable accuracy of theoretical predictions forvarious observables.

Few-nucleon systems with state-of-the-art chiral nucleon-nucleon forces