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The electronic ground state of Ca3LiOsO6 was recently considered within anintermediate coupling regime that revealed J=3/2 spin-orbit entangled magneticmoments. Through inelastic neutron scattering and density functional theory weinvestigate the magnetic interactions and probe how the magnetism is influencedby the change in hierarchy of interactions as we move from Ca3LiOsO6 (5d3) toCa3LiRuO6 (4d3). An alteration of the spin-gap and ordered local moment isobserved, however the magnetic structure, Neel temperature and exchangeinteractions are unaltered. To explain this behavior it is necessary to includeboth spin-orbit coupling and hybridization, indicating the importance of anintermediate coupling approach when describing 5$d$ oxides.

Interplay of spin-orbit coupling and hybridization in Ca3LiOsO6 and Ca3LiRuO6