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There have been continuous efforts in searching for unconventionalsuperconductivity over the past five decades. Compared to the well-establishedd-wave superconductivity in cuprates, the existence of superconductivity withother high-angular-momentum pairing symmetries is less conclusive. Bi/Niepitaxial bilayer is a potential unconventional superconductor with broken timereversal symmetry (TRS), for that it demonstrates superconductivity andferromagnetism simultaneously at low temperatures. We employ a speciallydesigned superconducting quantum interference device (SQUID) to detect, on theBi/Ni bilayer, the orbital magnetic moment which is expected if the TRS isbroken. An anomalous hysteretic magnetic response has been observed in thesuperconducting state, providing the evidence for the existence of chiralsuperconducting domains in the material.

Observation of Anomalous Magnetic Moments in Superconducting Bi/Ni Bilayer