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We show that evolution of magnetic properties in FeS under pressure cannot beexplained only in terms of a spin state transition. While uniform compressiondoes show substantial suppression of the local magnetic moment and increase ofthe weights of configurations with low spin, analysis of the local spin-spincorrelation function demonstrates increase of the spin itinerancy. This isrelated to a strong modification of the electronic structure under pressure: inthe high-pressure phase FeS is in the Fermi-liquid state, while decrease of thepressure moves the system to an orbital-selective regime.

Suppression of magnetism under pressure in FeS: a LDA+DMFT study