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Polarization selectivity of light-field-induced charge localization wasinvestigated in an organic metal alpha-(BEDT-TTF)2I3 with a triangular lattice.Dependences of transient reflectivity spectra on polarizations of the 7-fs pumpand probe lights indicate that a short-range charge order (CO) is efficientlyinduced from the metallic phase for the pump polarization perpendicular to the1010-type CO axis. Numerical solution of a time-dependent Schrodinger equationclarified that the 1010-CO is induced by field-induced re-distribution ofcharges cooperating with competing inter-site Coulomb repulsions in thetriangular lattice.

Polarization selectivity of charge localization induced by 7-fs nearly single-cycle light-field in an organic metal