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In Sr2NiIrO6, a metastable compound, the magnetic structure could be elucidated. The magnetic susceptibility data of the compound suggests a three-dimensional Heisenberg behavior. Moreover, neutron diffraction reveals a novel incommensurate magnetic order, requiring exchange interactions beyond second neighbor to stabilize this phase. An incommensurate propagation vector of k = (0, k, k) with k = 0.356 was observed in such a pseudocubic system. This can be an example of how to induce an incommensurate ground state and a possible type-II multiferroicity in double perovskites.

physical review. b./physical review. b

Incommensurate magnetic order in a quasicubic structure of the double-perovskite compound <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>Sr</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi>NiIrO</mml:mi><mml:mn>6</mml:mn></mml:msub></mml:mrow></mml:math>

Incommensurate magnetic order in a quasicubic structure of the double-perovskite compound Sr2NiIrO6