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We present a de Haas-van Alphen study of the Fermi surface of the lowtemperature antiferromagnet CeZn11 and its non-magnetic analogue LaZn11,measured by torque magnetometry up to fields of 33T and at temperatures down to320 mK. Both systems possess similar de Haas-van Alphen frequencies, with threeclear sets of features - ranging from 50T to 4kT - corresponding to three bandsof a complex Fermi surface, with an expected fourth band also seen weakly inCeZn11. The effective masses of the charge carriers are very light (<1 me) inLaZn11 but a factor of 2 - 4 larger in CeZn11, indicative of strongerelectronic correlations. We perform detailed density functional theory (DFT)calculations for CeZn11 and find that only DFT+U calculations with U=1.5 eV,which localize the 4f states, provide a good match to the measured de Haas-vanAlphen frequencies, once the presence of magnetic breakdown orbits is alsoconsidered. Our study suggests that the Fermi surface of CeZn11 is very closeto that of LaZn11 being dominated by Zn 3d, as the Ce 4f states are localisedand have little influence on its electronic structure, however, they areresponsible for its magnetic order and contribute to enhance electroniccorrelations.

A de Haas van Alphen study of the role of 4f electrons in antiferromagnetic CeZn11 as compared to its non-magnetic analogue LaZn11