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Competing orders widely exist in many material systems, such as superconductivity, magnetism, and ferroelectricity. LaCrSb3 is a highly anisotropic magnetic material in which the spins are aligned ferromagnetically (FM) in one direction and canted antiferromagnetically (AFM) in another in the Cr-Sb chains. Hole-doping with Sr and Ca in the La site suppresses the AFM correlations and transforms the anisotropic magnetic order into a FM lattice in all directions. First-principles density functional theory calculations show that the canted magnetic order becomes energetically less favorable compared to the FM order upon hole doping. Doping in the La site is an effective approach to modulate the competing orders in LaCrSb3. PACS number(s): 75.50.Cc, 75.50.Ee, 75.30.Cr, 75.30.Gw

physical review. b./physical review. b

From complex magnetism ordering to simple ferromagnetism in two-dimensional<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>LaCrS</mml:mi><mml:msub><mml:mi mathvariant="normal">b</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:math>by hole doping

From complex magnetism ordering to simple ferromagnetism in two-dimensionalLaCrSb3by hole doping