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We present an experimental and theoretical study of the optically detectedmagnetic resonance signals for ensembles of negatively charged nitrogen-vacancy(NV) centers in 13C isotopically enriched single-crystal diamond. We observefour broad transition peaks with superimposed sharp features at zero magneticfield and study their dependence on applied magnetic field. A theoretical modelthat reproduces all qualitative features of these spectra is developed.Understanding the magnetic-resonance spectra of NV centers in isotopicallyenriched diamond is important for emerging applications in nuclear magneticresonance.

Optically Detected Magnetic Resonances of Nitrogen-Vacancy Ensembles in 13C Enriched Diamond