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Superconducting FeSe single crystals of (001) orientation are synthesized viaa hydrothermal ion-release route. An Ising spin-nematic order is identified byour systematic measurements of in-plane angular-dependent magnetoresistance(AMR) and static magnetization. The turn-on temperature of anisotropic AMRsignifies the Ising spin-nematic ordering temperature Tsn, below which atwo-fold rotational symmetry is observed in the iron plane. A downwardcurvature appears below Tsn in the temperature dependence of staticmagnetization for the weak in-plane magnetic field as reported previously.Remarkably, we find a universal linear relationship between Tc and Tsn amongvarious superconducting samples, indicating that the spin nematicity and thesuperconductivity in FeSe have a common microscopic origin.

Observation of Ising spin-nematic order and its close relationship to the superconductivity in FeSe single crystals