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Monosilicides of 3d-metals frequently show a chiral magnetic ordering withthe absolute configuration defined by the chirality of the crystal structureand the sign of the Dzyaloshinskii-Moriya interaction (DMI). Structural andmagnetic chiralities are probed here for Fe$_{1-x}$Co$_x$Si series and theirmutual relationship is found to be dependent on the chemical composition. Thechirality of crystal structure was previously shown to be governed by crystalgrowth, and the value of the DMI is nearly the same for all monosilicides ofFe, Co and Mn. Our findings indicate that the sign of the DMI inFe$_{1-x}$Co$_x$Si is controlled by the Co composition $x$, thus, opening aroute towards controlled design of chiral spintronics devices.

physical review. b, condensed matter and materials physics

The Dzyaloshinskii-Moriya interaction is under control: an orchestrated  flip of the chiral link between structure and magnetism for  Fe$_{1-x}$Co$_x$Si