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Using dc and ac magnetometry, the pressure dependence of the magnetization ofthe three-dimensional antiferromagnetic coordination polymerMn(N(CN)$_{2}$)$_{2}$ was studied up to 12 kbar and down to 8K. The magnetictransition temperature, $T_c$, increases dramatically with applied pressure$(P)$, where a change from $T_c(P=\text{ambient}) = 16.0$ K to$T_c(P=12.1$~kbar$) = 23.5$ K was observed. In addition, a marked difference inthe magnetic behavior is observed above and below 7.1 kbar. Specifically, for$P<7.1$ kbar, the differences between the field-cooled and zero-field-cooled(fc-zfc) magnetizations, the coercive field, and the remanent magnetizationdecrease with increasing pressure. However, for $P>7.1$ kbar, the behavior isinverted. Additionally, for $P>8.6$ kbar, minor hysteresis loops are observed.All of these effects are evidence of the increase of the superexchangeinteraction and the appearance of an enhanced exchange anisotropy with appliedpressure.

Pressure-Induced Enhancement of the Magnetic Anisotropy in Mn(N(CN)$_{2}$)$_{2}$