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Under the terms of the Creative Commons Attribution License 3.0 (CC-BY).-- et al.We present a comprehensive study of the magnetism and morphology of an ultrahigh density array of Co nanoclusters self-assembled on the single atomic layer GdAu2 on Au(111) template surface. Combining scanning tunneling microscopy, x-ray magnetic circular dichroism, and magneto-optical Kerr effect measurements, we reveal a significant enhancement of the perpendicular magnetic anisotropy energy for noncoalesced single atomic layer nanoclusters compared to Co/Au(111). For coverages well beyond the onset of coalescence, we observe room-temperature in-plane magnetic remanence.We acknowledge funding from the Swiss National Science Foundation, from the Sino-Swiss Science and Technology Cooperation Project No. IZLCZ2 123892, from the Spanish Ministerio de Ciencia e Innovacion (MAT2010-21156-C03-03), from the Gipuzkoako Foru Aldundia, from the European Social Fund within the program\udJAE-Doc, the Basque Government (IT-621-13 and IT-627-13) and SAIOTEK (S-PE12UN095), as well as from the EU Calipso program for synchrotron access funding. The MBE chamber on DEIMOS was funded by the Agence National de\udla Recherche with Grant No. ANR-05-NANO-073.Peer Reviewe

physical review b

Magnetism and morphology of Co nanocluster superlattices on<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mrow><mml:mi mathvariant="normal">GdAu</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:math>/Au(111)–<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mo>(</mml:mo><mml:mn>13</mml:mn><mml:mo>×</mml:mo><mml:mn>13</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:math>

Magnetism and morphology of Co nanocluster superlattices onGdAu2/Au(111)–(13×13)