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Copyright © 2014 American Physical SocietyUsing the examples of laser-induced spin-reorientation phase transitions in TmFeO3 and ErFeO3 orthoferrites, we demonstrate that terahertz emission spectroscopy can obtain novel information about ultrafast laser-induced spin dynamics, which is not accessible by more common all-optical methods. The power of the method is evidenced by the fact that, in addition to the expected quasi-ferromagnetic and quasi-antiferromagnetic modes of the iron sublattices, terahertz emission spectroscopy enables detection of a resonance optically excited at an unexpected frequency of ∼0.3–0.35 THz. By recording how the amplitude and phase of the excited oscillations depend on temperature and applied magnetic field, we show that the unexpected mode has all the features of a spin resonance of the Fe3+ ions. We suggest that it can be assigned to transitions between the multiplet sublevels of the 6A1 ground state of the Fe+3 ions occupying rare-earth positions.European Commission's 7th Framework Program (FP7/2007–2013)Engineering and Physical Sciences Research Council (EPSRC)Netherlands Organization for Scientific Research (NWO)Foundation for Fundamental Research on Matter (FOM)ERCRussian GovernmentRFB

physical review b

Terahertz emission spectroscopy of laser-induced spin dynamics in<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi>TmFeO</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:math>and<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi>ErFeO</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:math>orthoferrites

Terahertz emission spectroscopy of laser-induced spin dynamics inTmFeO3andErFeO3orthoferrites