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We present here an investigation of the magnetic ordering in the Mott insulating oxyselenide materials Ln2O2Fe2OSe2 (Ln = Ce, Nd). Neutron powder diffraction data are consistent with a non-collinear multi-k ordering on the iron sublattice structure and analysis indicates a reduced magnetic correlation length perpendicular to the [Fe2O]2+ layers. The magnetic role of the Ln3+ cations is investigated and Ce3+ moments are found to order for T < 16 K.

physical review b

Structural and magnetic characterization of iron oxyselenides<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi>Ce</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi mathvariant="normal">Fe</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi mathvariant="normal">OSe</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>and<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:…

Structural and magnetic characterization of iron oxyselenidesCe2O2Fe2OSe2and