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The Jeff=1/2 state is manifested in systems with large cubic crystal fieldsplitting and spin-orbit coupling that are comparable to the on-site Coulombinteraction, U. 5d transition metal oxides host parameters in this regime andstrong evidence for this state in Sr2IrO4, and additional iridates, has beenpresented. All the candidates, however, deviate from the cubic crystal fieldrequired to provide an unmixed canonical Jeff=1/2 state, impacting thedevelopment of a robust model of this novel insulating and magnetic state. Wepresent results that not only show Ca4IrO6 hosts the state, but furthermoreuniquely resides close to the ideal case required for an unmixed Jeff=1/2state.

Jeff=1/2 Mott spin-orbit insulating state close to the cubic limit in Ca4IrO6