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Nanomagnetometry using the nitrogen-vacancy (NV) centre in diamond hasattracted a great deal of interest because of the combined features of roomtemperature operation, nanoscale resolution and high sensitivity. One of theimportant goals for nano-magnetometry is to be able to detect nanoscale nuclearmagnetic resonance (NMR) in individual molecules. Our theoretical analysisshows how a single molecule at the surface of diamond, with characteristic NMRfrequencies, can be detected using a proximate NV centre on a time scale oforder seconds with nanometer precision. We perform spatio-temporal resolutionoptimisation and also outline paths to greater sensitivity. In addition, themethod is suitable for application in low and relatively inhomogeneousbackground magnetic fields in contrast to both conventional liquid and solidstate NMR spectroscopy.

Single molecule NMR detection and spectroscopy using single spins in diamond