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We report the first observation of Shubnikov-de Haas (SdH) oscillations andquantized Hall resistance in the multilayered massless Dirac fermion system$\alpha$-(BEDT-TTF)$_2$I$_3$ with tilted cones. Holes were injected into thethin crystal fixed on a polyethylene naphthalate (PEN) substrate by contactelectrification. The detection of SdH oscillations whose phase was modified byBerry's phase $\pi$ strongly suggested that the carrier doping was successfulin this system. We succeeded in detecting the quantum Hall effect (QHE) withthe steps which is the essence of two dimensional Dirac fermion systems. Thenumber of effectively doped layers was examined to be two in this device. Wereveal that the correlation between effective layers plays an important role inQHE.

Quantum Hall effect in multilayered massless Dirac fermion systems with tilted cones