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We report nuclear magnetic resonance data in the bilayer nickelate La3Ni2O6.This material belongs to a family of low valence nickel oxides with squareplanar coordination of the Ni ions and is isoelectronic to the high temperaturesuperconducting cuprates. Although the three layer nickelate compound exhibitsa spin-state transition accompanied by antiferromagnetic order, the bilayermaterial shows no phase transition. The NMR data in the bilayer La3Ni2O6 revealthe presence of antiferromagnetic spin fluctuations down to 5K that aresurprisingly similar to those present in the magnetically ordered trilayerLa4Ni3O8, suggesting a similar electronic structure in the paramagnetic phaseof both compounds.

NMR evidence for spin fluctuations in the bilayer nickelate La3Ni2O6