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Due of its polymorphism, Mn$_2$FeSbO$_6$ can be synthesized at high pressuresand temperatures as a ferrimagnetic ilmenite or an antiferromagneticperovskite. The structural phase transformation is discussed in detail, andmagnetic structures are proposed for both phases. The high-pressureMn$_2$FeSbO$_6$ polymorph is a rare example of $A_2 B'B"$O$_6$ perovskite withsolely Mn cations on the $A$-site. Fe and Sb cations are ordered on the$B$-sites. Theoretical calculations for the perovskite phase suggest a complexmagnetic structure, holding an electronic polarization.

Mn$_2$FeSbO$_6$: a ferrimagnetic ilmenite and an antiferromagnetic perovskite