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Magnetic properties in the quasi-one-dimensional organic salt (TMTTF)2SbF6are investigated by 13C NMR under pressures. Antiferromagnetic phase transitionat ambient pressure (AFI) is confirmed. Charge-ordering is suppressed bypressure and is not observed under 8 kbar. For 5 < P < 20 kbar, a sharpspectrum and the rapid decrease of the spin-lattice relaxation rate 1/T1 wereobserved below about 4 K, attributed to a spin-gap transition. Above 20 kbar,extremely broadened spectrum and critical increase of 1/T1 were observed. Thisindicates that the system enters into another antiferromagnetic phase (AFII)under pressure. The slope of the antiferromagnetic phase transition temperatureT_AFII, dT_AFII/dP, is positive, while T_AFI decreases with pressure. Themagnetic moment is weakly incommensurate with the lattice at 30 kbar.

13C NMR study of the magnetic properties of the quasi-one-dimensional conductor, (TMTTF)2SbF6