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Using Kubo's linear response theory, we derive expressions for thefrequency-dependent electrical conductivity (Kubo-Greenwood formula),thermopower, and thermal conductivity in a strongly correlated electron system.These are evaluated within ab initio molecular dynamics simulations in order tostudy the thermoelectric transport coefficients in dense liquid hydrogen,especially near the nonmetal-to-metal transition region. We also observesignificant deviations from the widely used Wiedemann-Franz law which isstrictly valid only for degenerate systems and give an estimate for its validscope of application towards lower densities.

Electronic transport coefficients from ab initio simulations and application to dense liquid hydrogen