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We report the remarkably robust ferroelectric state in the multiferroiccompound Mn$_{1-x}$Zn$_x$WO$_4$. The substitution of the magnetic Mn$^{2+}$with nonmagnetic Zn$^{2+}$ reduces the magnetic exchange and provides controlof the various magnetic and multiferroic states of MnWO$_4$. Only 5 % of Znsubstitution results in a complete suppression of the frustrated collinear(paraelectric) low temperature phase. The helical magnetic and ferroelectricphase develops as the ground state. The multiferroic state is stable up to ahigh level of substitution of more than 50 %. The magnetic, thermodynamic, anddielectric properties as well as the ferroelectric polarization of singlecrystals of Mn$_{1-x}$Zn$_x$WO$_4$ are studied for different substitutions upto x=0.5. The magnetic phases have been identified in single crystal neutronscattering experiments. The ferroelectric polarization scales with the neutronintensity of the incommensurate peak of the helical phase.

Robust Ferroelectric State in Multiferroic Mn$_{1-x}$Zn$_x$WO$_4$