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The magnetic and multiferroic phase diagram of Mn$_{0.85}$Co$_{0.15}$WO$_4$single crystals is investigated by means of magnetic, heat capacity,dielectric, polarization, and neutron scattering experiments. Three magneticphase transitions are detected through distinct anomalies in all physicalquantities. The ferroelectric polarization is observed only along the b-axisbelow 10 K but not along the a-axis as recently suggested. The magnetic phasesstudied by neutron scattering are very complex. Up to four different magneticstructures, partially coexisting at certain temperature ranges, have beenidentified. Upon decreasing temperature two commensurate phases (AF4, AF1) arefollowed by an incommensurate phase (AF5) and a second incommensurate phase(AF2) is detected as a minor phase. The ferroelectric polarization is possiblyassociated with both (AF2 and AF5) phases.

Magnetic and multiferroic phases of single-crystalline Mn$_{0.85}$Co$_{0.15}$WO$_4$