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The effect of high pressure (0 - 8 GPa) on the magnetic structure ofpolycrystalline samples of La0.5Ca0.5-xSrxMnO3 (0.1 -< x -< 0.4) manganites at5 K is investigated using neutron diffraction technique. Application ofpressure is found to modify the previously reported magnetic structure,observed under ambient conditions, in these compounds [I. Dhiman et al., Phys.Rev. B 77, 094440 (2008)]. In x = 0.1 composition, at 4.6(2) GPa and beyond,A-type antiferromagnetic structure is found to coexist with CE-typeantiferromagnetic phase, observed at ambient pressure, with TN ~ 150 K. For x =0.3 sample, as a function of pressure the CE-type phase is fully suppressed at2.3(1) GPa and A-type antiferromagnetic phase is favored. Further Sr doping atx = 0.4, the A-type antiferromagnetic phase is observed at ambient pressure andfor T < TN (~ 250K). This phase is retained in the studied pressure range.However, the magnetic moment progressively reduces with increasing pressure,indicating the suppression of A-type antiferromagnetic phase. The present studybrings out the fragile nature of the CE-type antiferromagnetic state in halfdoped manganites as a function of pressure and disorder \sigma 2. We observethat pressure required for destabilizing the CE-type antiferromagnetic state isreduced with increasing disorder \sigma 2. External pressure and changingA-site ionic radii have analogous effect on the magnetic structure.

Pressure effects on the magnetic structure in La0.5Ca0.5-xSrxMnO3 (0.1 -< x -< 0.4) manganites