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Pulsed field magnetization experiments extend the typical metamagneticstaircase of CuFeO2 up to 58 T to reveal an additional first order phasetransition at high field for both the parallel and perpendicular fieldconfiguration. Virtually complete isotropic behavior is retrieved only abovethis transition, indicating the high-field recovery of the undistortedtriangular lattice. A consistent phenomenological rationalization for the fielddependence and metamagnetism crossover of the system is provided, demonstratingthe importance of both spin-phonon coupling and a small field-dependenteasy-axis anisotropy in accurately describing the magnetization process ofCuFeO2.

High-field recovery of the undistorted triangular lattice in the frustrated metamagnet CuFeO2