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Using different experimental techniques combined with density functionalbased theoretical methods we have explored the formation ofinterface-stabilized manganese oxide structures grown on Pd(100) at(sub)monolayer coverage. Amongst the multitude of phases experimentallyobserved we focus our attention on four structures which can be classified intotwo distinct regimes, characterized by different building blocks. Twooxygen-rich phases are described in terms of MnO(111)-like O-Mn-O trilayers,whereas the other two have a lower oxygen content and are based on aMnO(100)-like monolayer structure. The excellent agreement between calculatedand experimental scanning tunneling microscopy images and vibrational electronenergy loss spectra allows for a detailed atomic description of the exploredmodels.

Structural and vibrational properties of two-dimensional $\rm Mn_xO_y$ nanolayers on Pd(100)