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We studied the temperature stability of the endohedral fullerene molecule,N@C60, inside single-wall carbon nanotubes using electron spin resonancespectroscopy. We found that the nitrogen escapes at higher temperatures in theencapsulated material as compared to its pristine, crystalline form. Thetemperature dependent spin-lattice relaxation time, T_1, of the encapsulatedmolecule is significantly shorter than that of the crystalline material, whichis explained by the interaction of the nitrogen spin with the conductionelectrons of the nanotubes.

Enhanced thermal stability and spin-lattice relaxation rate of N@C60 inside carbon nanotubes