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We present a study on the structural, spectroscopic, conducting, \udand\udmagnetic properties of Mg5C60, which is a two-dimensional (2D)\udfulleride polymer. The polymer phase is stable up to the \udexceptionally\udhigh temperature of 823 K. The infrared and Raman studies \udsuggest the\udformation of single bonds between the fulleride ions and \udpossibly\udMg-C-60 covalent bonds. Mg5C60 is a metal at ambient \udtemperature, as\udshown by electron spin resonance and microwave conductivity\udmeasurements. The smooth transition from a metallic to a \udparamagnetic\udinsulator state below 200 K is attributed to Anderson \udlocalization\uddriven by structural disorder

physical review b

Structure and properties of the stable two-dimensional conducting polymer<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="normal">Mg</mml:mi><mml:mn>5</mml:mn></mml:msub><mml:msub><mml:mi mathvariant="normal">C</mml:mi><mml:mn>60</mml:mn></mml:msub></mml:mrow></mml:math>

Structure and properties of the stable two-dimensional conducting polymerMg5C60