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Tweaking the properties of carbon nanotubes is a prerequisite for theirpractical applications. Here we demonstrate fine-tuning the electronicproperties of single-wall carbon nanotubes via filling with ferrocenemolecules. The evolution of the bonding and charge transfer within the tube isdemonstrated via chemical reaction of the ferrocene filler ending up assecondary inner tube. The charge transfer nature is interpreted well withindensity functional theory. This work gives the first direct observation of afine-tuned continuous amphoteric doping of single-wall carbon nanotubes.

Fine-tuning the functional properties of carbon nanotubes via the interconversion of encapsulated molecules