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Magnetic properties of the silver vanadium phosphate Ag(2)VOP(2)O(7) arestudied by means of magnetic susceptibility measurements and electronicstructure calculations. In spite of the layered crystal structure suggesting 1Dor 2D magnetic behavior, this compound can be understood as a spin dimersystem. The fit of the magnetic susceptibility indicates an intradimerinteraction of about 30 K in perfect agreement with the computational results.Our study emphasizes the possible pitfalls in interpreting experimental data onstructural basis only and points out the importance of microscopic models forthe understanding of the magnetic properties of vanadium phosphates.

Magnetic properties of Ag(2)VOP(2)O(7): an unexpected spin dimer system