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Raman spectra of thin solid electrolyte films obtained by sputtering alithium sulfate target in nitrogen plasma are measured and compared to abinitio electronic structure calculations for clusters composed of 28 atoms.Agreement between measured and calculated spectra is obtained when oxygen atomsare replaced by nitrogen atoms and when the nitrogen atoms form bonds with eachother. This suggests that the incorporation of nitrogen during the sputteringprocess leads to structures in the film, which prevent crystallization of thesethin film salt glasses.

Structure of glassy lithium sulfate films sputtered in nitrogen (LISON): Insight from Raman spectroscopy and ab initio calculations