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Size-selected silver clusters on Ag(111) were fabricated with the tip of ascanning tunneling microscope. Unoccupied electron resonances give rise toimage contrast and spectral features which shift toward the Fermi level withincreasing cluster size. Linear assemblies exhibit higher resonance energiesthan equally sized compact assemblies. Density functional theory calculationsreproduce the observed energies and enable an assignment of the resonances tohybridized atomic 5s and 5p orbitals with silver substrate states.

Unoccupied states of individual silver clusters and chains on Ag(111)